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Alioune started his career in industry with Pechiney and then joined Sonatel in 1988, first working on management control then as Chief Financial Officer. In 2002 he was appointed CEO of Ikatel in Mali which became Orange Mali and which he lead for 10 years. In 2012 he was promoted CEO of Sonatel, member company of the Orange group in Senegal, and the reference operator in West Africa. Sonatel is present in Senegal, Mali, Guinea, Guinea Bissau and Sierra Leone.
Since 2nd May 2018, Alioune is the CEO of Orange Middle East and Africa.